Art in Biosynthesis. The Synthetic Chemist's Challenge by Darshan Ranganathan

By Darshan Ranganathan

The publication initiatives Nature as an natural chemist preferrred, and offers consultant examples whose biosynthetic pathways are recognized at the foundation of experimentation.

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Amer. Chem. , 88, 4750 (1966); E. J. Corey, P. R. Ortiz de Montellano, K. Lin and P. D. G. Dean, J. Amer. Chem. , _§£, 2797 (1967); E. E. van Tamelen, J. D. Willett, R. B. Clayton, and K. E. Lord, J. Amer. Chem. S o c , _88, 4752 (1966); E. E. van Tamelen, J. D. Willett and R. B. Clayton, J. Amer. Chem S o c , 8»9, 3371 (I967) . 5. The formation of this intermediate from squalene epoxide requires the generation of a comparatively unstable ring B boat in intermediate generated by chair-boat-chair cyclisation.

24l, 5276 (1966)). 9. Magnesium protoporphyrin monômethyl ester is found in some chlorophyll deficient mutants of Chlorella (S. Graniek, J. biol. , 236, ll68 (1961)) and wild type R. sphéroïdes (0. T. G. Jones, Biochem. , 86, 429 (1963)). The enzyme 52 CHLOROPHYLL system that carries out the methylation of magnesium protoporphyrin was characterised as S-adenosyl methioninemagnesium protoporphyrin methyl transferase; the methyl group donor was found to be S-adenosyl methionine (K. D. Gibson, A.

243, 4966 (I968); A. C. Swindell and J. L. , p. 55^6; N. J. Moir, W. L. Miller, and J. L. Gaylor, Biochem. Biophys. Res. , _33, 916 (1968); W. L. Miller and J. L. Gaylor, J. Biol. , 245, 5369, 5375 (1970); G. M. Hornby and G. S. Boyd, Biochem. Biophys. Res. , 40, 1452 (1970); K. B. Sharpless, T. E. Snyder, T. A. Spencer, K. K. Maheshwari, J. A. Nelson, and R. B. Clayton, J. Amer. Chem. , 91, 3394 (I969)). 57 CHOLESTEROL o 9. The transposition ted to take place Biochem. , Il43 Dempsey, J. Biol.

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Art in Biosynthesis. The Synthetic Chemist's Challenge by Darshan Ranganathan
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